Accelerators integrated on-die with General-Purpose CPUs (GP-CPUs) can yield significant performance and power improvements. Their extensive use, however, is ultimately limited by their area overhead; due to their high degree of specialization, the opportunity cost of investing die real estate on accelerators can become prohibitive, especially for general-purpose architectures. In this paper we present a novel technique aimed at mitigating this opportunity cost by allowing GP-CPU cores to reuse accelerator memory as a non-uniform cache architecture (NUCA) substrate. On a system with a last level-2 cache of 128kB, our technique achieves on average a 25% performance improvement when reusing four 512 kB accelerator memory blocks to form a level-3 cache. Making these blocks reusable as NUCA slices incurs on average in a 1.89% area overhead with respect to equally-sized ad hoc cache slices.